Zimbabwe hosts Africa's largest hard-rock lithium reserves, presenting a significant opportunity for local battery-grade lithium production. This study focuses on optimizing froth flotation for sustainable beneficiation of spodumene and lepidolite, primarily from the Bikita lithium deposit. Experimental results confirmed froth flotation as a highly effective method, achieving Li₂O concentrate grades up to 5.8% from ores initially averaging 1–3.2% Li₂O. Anionic collectors such as oleic acid and sodium oleate were evaluated, with oleic acid proving more effective for spodumene and sodium oleate for lepidolite. Optimal flotation conditions included particle sizes of 45–90 microns, a pH of 10, and a collector dosage of 250 mg/L. Recovery rates exceeded 90%, highlighting froth flotation's potential for high-efficiency, battery- grade lithium recovery in Zimbabwe.